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E-grāmata: Mechanochemistry in Materials

Edited by (University of Southern Mississippi, USA), Edited by (Duke University, USA)
  • Formāts: 196 pages
  • Sērija : Polymer Chemistry Series Volume 26
  • Izdošanas datums: 24-Oct-2017
  • Izdevniecība: Royal Society of Chemistry
  • Valoda: eng
  • ISBN-13: 9781782623885
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Mechanochemistry in MaterialsPalielināt
  • Formāts: 196 pages
  • Sērija : Polymer Chemistry Series Volume 26
  • Izdošanas datums: 24-Oct-2017
  • Izdevniecība: Royal Society of Chemistry
  • Valoda: eng
  • ISBN-13: 9781782623885
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Mechanochemistry in materials science has experienced tremendous growth in the last 5 years and has developed to become one of the most important topics in polymer science today.

With tremendous growth over the last five years, mechanochemistry has become one of the most important topics in current polymer science research. With a particular focus on polymers and soft materials, Mechanochemistry in Materials looks at the subject from the application of macroscopic forces to solid systems of macroscopic dimensions.

The book has been divided according to length scale covering both experimental and theoretical considerations simultaneously. The first section of the book focuses on inspiration from nature, exploring and explaining multiple biological phenomena. The second section discusses molecular mechanochemistry, including the theoretical understanding of the transduction of mechanical force and its impact on covalent bonds cleavage and formation. The final section considers the implementation of these phenomena at the mesoscale and discusses the use of supramolecular/reversible aspects with similarities to biological systems.

The book provides a unique comparison with natural systems and contains all the important achievements in the area from the last decade. Appealing to a broad range of materials scientists, working in industry and academia, this well-presented and comprehensive title will be essential reading for researchers.

Chapter 1 Mechanochemistry: Inspiration from Biology
1(35)
Tamuka Chidanguro
Wengui Weng
Yoan C. Simon
1.1 Introduction and Historical Perspective
1(2)
1.2 Biomimetism and Rationale for Emulating Mechanotransduction Pathways
3(12)
1.2.1 Principles of Biomimetism and Strategies to Implement It
3(1)
1.2.2 Introduction of the Importance of Mechanotransduction Pathways for Living Organisms
4(2)
1.2.3 Adaptivity in Bones
6(9)
1.3 Sensing
15(15)
1.3.1 Via Protein Unfolding
15(6)
1.3.2 Via Ion Channel Opening
21(9)
1.4 Conclusion
30(6)
References
31(5)
Chapter 2 Mechanophores for Chemical Function
36(17)
C. E. Diesendruck
2.1 Introduction
36(1)
2.2 Creation of Reactive Species
37(5)
2.2.1 Radicals
37(1)
2.2.2 Carbon Cations
38(1)
2.2.3 Reactive Organic Functional Groups
39(3)
2.3 Catalyst Activation
42(2)
2.4 Spectral Change
44(3)
2.5 Production of Small Molecules
47(1)
2.6 Other
48(1)
2.7 Conclusions and Perspectives
49(4)
References
50(3)
Chapter 3 Optical Sensing of Stress in Polymers
53(23)
R. Gostl J. M. Clough
R. P. Sijbesma
3.1 Introduction
53(2)
3.2 Bond--Isomerization Reactions
55(3)
3.3 Covalent Bond Scission Reactions
58(5)
3.4 Conjugated Polymers
63(1)
3.5 Chromophore Rearrangement
64(3)
3.6 Photonic Polymers and Cholesteric Liquid Crystals
67(2)
3.7 Conclusion
69(7)
Acknowledgements
70(1)
References
70(6)
Chapter 4 Materials Design Principles for Mechanochemical Transduction
76(43)
M. N. Silberstein
M. S. Manivannan
4.1 Introduction
76(1)
4.2 Mechanics Terminology
77(2)
4.3 Mechanophore Kinetics
79(3)
4.4 Experimental Techniques for MCR Polymers
82(5)
4.5 Elastomers
87(12)
4.6 Glassy Polymers
99(8)
4.7 Composites and Coatings
107(1)
4.8 Mechanochemically Modified Networks
108(5)
4.9 Conclusions
113(6)
Abbreviations
114(1)
Acknowledgements
115(1)
References
115(4)
Chapter 5 Tailoring Mechanochemical Reactivity of Covalent Bonds in Polymers by Non-covalent Interactions
119(36)
Huan Zhang
Linxing Zhang
Yinjun Chen
Yangju Lin
Wengui Weng
5.1 Introduction
119(1)
5.2 Theoretical Background of Polymer Mechanochemistry and the Effects of Supramolecular Interactions
120(5)
5.2.1 Coil-to-stretch Transition and Bead-rod Model
120(1)
5.2.2 Intra-chain Non-covalent Interactions
121(2)
5.2.3 Inter-chain Non-covalent Interactions
123(2)
5.2.4 Non-covalent Interactions in the Bulk
125(1)
5.3 Experimental Observations
125(18)
5.3.1 Mechanical Cleavage of Covalent Bonds in Dilute Solution
125(5)
5.3.2 Effects of Strong Hydrogen Bonding Interactions on the Activation of Mechanophores in the Bulk
130(6)
5.3.3 Effects of Van de Waals Interactions
136(4)
5.3.4 Effect of Metallo-supramolecular Interactions
140(3)
5.4 Non-covalent Interactions in Stress-responsive Materials
143(3)
5.4.1 Activation of Mechanophores and Irreversible Deformation of the Matrix
143(1)
5.4.2 Successive Mechanochemical Activation in Hydrogen-bonded Reinforced Elastomers
143(3)
5.5 Conclusions and Outlook
146(9)
5.5.1 Conclusions
146(1)
5.5.2 Outlook
147(1)
Acknowledgements
147(1)
References
148(7)
Chapter 6 Mechanochemistry of Polymer Brushes
155(12)
Nariye Cavusoglu Ataman
Jan Genzer
Harm-Anton Klok
6.1 Introduction
155(1)
6.2 Degrafting of Polymer Brushes
156(8)
6.3 Summary and Conclusions
164(3)
References
165(2)
Chapter 7 Coupling Mechanics to Chemical Reactions to Create "Materials that Compute"
167(27)
Victor V. Yashin
Steven P. Levitan
Anna C. Balazs
7.1 Introduction
167(2)
7.2 Modeling Self-oscillating Gels
169(4)
7.2.1 Kinetics of the BZ Reaction in a Polymer Gel
169(2)
7.2.2 Gel Swelling in the Presence of an External Force
171(1)
7.2.3 Values of Parameters Used in the Calculations
172(1)
7.3 Modeling Force-controlled Entrainment of BZ Gels
173(8)
7.3.1 Phase Dynamics Equations for Mechanically Deformed BZ Gels
174(2)
7.3.2 Entraining the Responsive BZ Gel
176(5)
7.4 Self-oscillating Gels Coupled Through Piezoelectric Films
181(10)
7.5 Conclusions
191(3)
Acknowledgement
192(1)
References
192(2)
Subject Index 194
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