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Nanogap Electrodes [Hardback]

Edited by Tao Li (University of Copenhagen, Denmark)

Formāts: Hardback, 432 pages, height x width x depth: 240x170x170 mm, weight: 964 g
Izdošanas datums: 04-Aug-2021
Izdevniecība: Blackwell Verlag GmbH
ISBN-10: 3527332715
ISBN-13: 9783527332717

Citas grāmatas par šo tēmu:

Electronics engineering - (Noliktavā: 1 punkts)
Nanotechnology - (Noliktavā: 1 punkts)

Hardback
Cena: 159,99 €
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Bibliotēkām

Formāts: Hardback, 432 pages, height x width x depth: 240x170x170 mm, weight: 964 g
Izdošanas datums: 04-Aug-2021
Izdevniecība: Blackwell Verlag GmbH
ISBN-10: 3527332715
ISBN-13: 9783527332717

Citas grāmatas par šo tēmu:

Electronics engineering - (Noliktavā: 1 punkts)
Nanotechnology - (Noliktavā: 1 punkts)

Permanent link: https://www.kriso.lv/db/9783527332717.html

Keywords:

Unique in combining various synthesis strategies with applications for nanogap electrodes, this book introduces the topic before devoting whole sections to synthesis, characterization, and applications, finishing with interesting phenomena observed using molecular-based devices.

Unique in its scope, this book comprehensively combines various synthesis strategies with applications for nanogap electrodes. Clearly divided into four parts, the monograph begins with an introduction to molecular electronics and electron transport in molecular junctions, before moving on to a whole section devoted to synthesis and characterization. The third part looks at applications with single molecules or self-assembled monolayers, and the whole is rounded off with a section on interesting phenomena observed using molecular-based devices.

Preface

1 Nanogap Electrodes and Molecular Electronic Devices

(24)

Tao Li

1.1 Introduction

(1)

1.2 Overview of Molecular Electronics

(14)

1.2.1 Why Molecular Electronics

(1)

1.2.1.1 History of Computing

(3)

1.2.1.2 Moore's Law

(2)

1.2.1.3 Molecular Electronics: A Beyond-CMOS Option

(2)

1.2.2 Molecular Materials for Organic Electronics

(1)

1.2.2.1 OLEDs

(1)

1.2.2.2 OFETs

(1)

1.2.2.3 OPVs

(1)

1.2.3 Molecules for Molecular-Scale Electronics

(3)

1.3 Introduction to Nanogap Electrodes

(3)

1.4 Summary and Outlook

(6)

References

(6)

2 Electron Transport in Single Molecular Devices

(32)

Lei-Lei Nian

Liang Ma

Jing-Tao Lii

2.1 Introduction

(1)

2.2 General Methods

(1)

2.2 Transport Mechanisms

(5)

2.2.2 Nonequilibrium Green's Function Method

(3)

2.2.3 Master Equation Method

(2)

2.3 Single Electron Transport Through Single Molecular Junction

(4)

2.3.1 Coherent Transport

(1)

2.3.2 Hopping Transport

(3)

2.4 Effect of Many-Body Interactions

(13)

2.4.1 Electron-Vibration Interaction

(2)

2.4.1.1 Weak Coupling Regime

(3)

2.4.1.2 Strong-Coupling Regime

(3)

2.4.2 Electron-Electron Interaction

(1)

2.4.2.1 Coulomb Blockade

(2)

2.4.2.2 Kondo Effect

(3)

2.5 Thermoelectric Transport

(3)

2.6 First-Principles Simulations of Transport in Molecular Devices

(1)

2.7 Conclusions

(5)

References

(5)

3 Fabricating Methods and Materials for Nanogap Electrodes

(132)

Xianhui Huang

Weiqiang Zhang

Dong Xiang

Tao Li

3.1 Introduction

(2)

3.2 Mechanical Controllable Break Junctions

(9)

3.3 Electrochemical and Chemical Deposition Method

(7)

3.3.1 Electroplating and Feedback System

(6)

3.3.2 Chemical Deposition

(1)

3.4 Oblique Angle Shadow Evaporation

(3)

3.5 Electromigration and Electrical Breakdown Method

(11)

3.5.1 Device Fabrication

(3)

3.5.2 Gap Size Control

(2)

3.5.3 Electromigration Applications

(5)

3.6 Molecular Scale Template

(13)

3.6.1 Molecular Rulers

(5)

3.6.2 Inorganic Films as Templates

(2)

3.6.3 On-Wire Lithography

(4)

3.6.4 Nanowire Mask

100

(2)

3.7 Focused Ion Beam

102

(6)

3.8 Scanning Probe Lithography and Conducting Probe-Atomic Force Microscopy

108

(5)

3.8.1 Destructive Way

108

(3)

3.8.2 Constructive Way

111

(1)

3.8.3 Conducting Probe-Atomic Force Microscopy

112

(1)

3.9 Nanogap Electrodes Prepared with Nonmetallic Materials

113

(61)

3.9.1 Introduction

113

(1)

3.9.2 Nanogap Electrodes Made from Carbon Materials

114

(1)

3.9.2.1 Advantages of Carbon Materials

114

(1)

3.9.2.2 Carbon Nanotubes for Nanogap Electrodes

115

(15)

3.9.2.3 Graphene

130

(23)

3.9.2.4 Silicon Nanogap Electrodes

153

(18)

3.9.2.5 Other Materials

171

(3)

3.10 Summary and Outlook

174

(15)

References

175

(14)

4 Characterization Methods and Analytical Techniques for Nanogap Junction

189

(50)

Baiti Li

Ziyan Wang

Bin Han

Xi Yu

4.1 Current-Voltage Analysis

189

(17)

4.1.1 Coherent Tunneling Transport

190

(5)

4.1.2 Transition Voltage Spectroscopy

195

(3)

4.1.3 Incoherent Transport

198

(8)

4.2 Inelastic Tunneling Spectroscopy (IETS)

206

(20)

4.2.1 Principle and Measurement of IETS

206

(3)

4.2.2 Selection Rule and Charge Transport Pathway

209

(5)

4.2.3 Line Shape of the IETS

214

(4)

4.2.4 Application of the IETS

218

(1)

4.2.5 Mapping the Charge Transport Pathway in Protein Junction by IETS

219

(3)

4.2.6 STM Imaging by IETS

222

(4)

4.3 Optical and Optoelectronic Spectroscopy

226

(6)

4.4 Concluding Remarks

232

(7)

Appendix

233

(1)

References

234

(5)

5 Single-Molecule Electronic Devices

239

(62)

Shengxiong Xiao

5.1 Introduction

239

(1)

5.2 Wiring Molecules into "Gaps": Anchoring Groups and Assembly Methods

240

(12)

5.2.1 Anchor Groups

240

(5)

5.2.2 Effect of Anchor-Bridge Orbital Overlaps on Conductance

245

(5)

5.2.3 In Situ Chemical Reactions to Produce Covalent Contacts

250

(2)

5.3 Electrical Rectifier

252

(17)

5.3.1 Rectification Toward Diodes

255

(1)

5.3.2 General Mechanisms for Molecular Rectification

256

(1)

5.3.2.1 Aviram-Ratner Model

256

(1)

5.3.2.2 Kornilovitch-Bratkovsky-Williams Model

257

(1)

5.3.2.3 Datta-Paulsson Model

258

(1)

5.3.3 Rectification Originated from Molecules

259

(1)

5.3.3.1 D-σ-A and D-π-A Systems

259

(1)

5.3.3.2 D-A Diblock Molecular System

260

(4)

5.3.4 Rectification Stemming from Different Interfacial Coupling

264

(1)

5.3.4.1 Different Electrodes

264

(1)

5.3.4.2 Anchoring Groups

265

(1)

5.3.4.3 Contact Geometry

265

(1)

5.3.4.4 Interfacial Distance

266

(1)

5.3.5 Additional Molecular Rectifiers

267

(2)

5.4 Conductance Switches

269

(13)

5.4.1 Voltage Pulse Induced Switches

270

(1)

5.4.2 Light-Induced Switching

271

(4)

5.4.3 Switching Triggered by Chemical Process (Redox and pH)

275

(3)

5.4.4 Spintronics-Based Switch

278

(4)

5.5 Gating the Transport: Transistor-Like Single-Molecule Devices

282

(9)

5.5.1 Electrostatic Gate Control

282

(5)

5.5.2 Side Gating

287

(1)

5.5.3 Electrochemical Gate Control

288

(2)

5.5.4 Molecular Quantum Dots

290

(1)

5.6 Challenges and Outlooks

291

(10)

References

292

(9)

6 Molecular Electronic Junctions Based on Self-Assembled Monolayers

301

(44)

Yuqing Liu

Zhongming Wei

6.1 Introduction

301

(1)

6.2 Molecular Monolayers for Molecular Electronics Devices

302

(12)

6.2.1 Monolayers Covalently Bonded to Noble Metals

303

(6)

6.2.2 Monolayers Attached to Non-metal Substrates

309

(3)

6.2.3 Langmuir-Blodgett Method

312

(2)

6.3 Top Electrodes

314

(15)

6.3.1 Deposited Metal

314

(1)

6.3.1.1 Direct Evaporation

315

(1)

6.3.1.2 Indirect Evaporation

316

(3)

6.3.2 Make Top Contact by Soft Methods

319

(1)

6.3.2.1 Lift-and-Float Approach

319

(1)

6.3.2.2 Crosswire Junction

320

(2)

6.3.2.3 Transfer Printing

322

(1)

6.3.2.4 Graphene as Top Electrode

323

(3)

6.3.2.5 Liquid Metal Contact

326

(3)

6.4 Experimental Progress with Ensemble Molecular Junctions

329

(5)

6.5 Outlook

334

(11)

References

335

(10)

7 Toward Devices and Applications

345

(55)

Ajuan Cui

Kasper Norgaard

7.1 Introduction

345

(1)

7.2 Major Issues: Reliability and Robustness

346

(12)

7.2.1 Single Molecular Device

347

(1)

7.2.1.1 Top-Contact Junctions

347

(1)

7.2.1.2 Planar Metallic Nanogap Electrodes

347

(2)

7.2.1.3 Planar Nanogap Electrodes Based on Single Walled Carbon Nanotubes (SWCNTs) or Graphene

349

(1)

7.2.1.4 The Absorption of Molecule on the Surface of SWCNTs or Graphene

350

(1)

7.2.2 Molecular Device Based on Molecule Monolayer

351

(2)

7.2.2.1 Bottom Electrodes

353

(1)

7.2.2.2 Insulating Layer with Holes to Define the Size of the Bottom Electrodes

353

(1)

7.2.2.3 Molecule Monolayer Formation

354

(1)

7.2.2.4 Top Electrodes

354

(4)

7.3 Potential Integration Solutions

358

(13)

7.3.1 Carbon Nanotube or Graphene Interconnects

359

(5)

7.3.2 Self-Assembled Monolayers for Integrated Molecular Junctions

364

(4)

7.3.3 Cross Bar Architecture

368

(3)

7.4 Beyond Simple Charge Transport

371

(24)

7.4.1 Mechanics

371

(4)

7.4.2 Thermoelectronics

375

(6)

7.4.3 Quantum Interference

381

(5)

7.4.4 Spintronics

386

(1)

7.4.4.1 SAM-Based Magnetic Tunnel Junctions

386

(1)

7.4.4.2 Molecule Based Spin-Valves or Magnetic Tunnel Junctions

387

(2)

7.4.4.3 Single Molecular Spin Transistor

389

(2)

7.4.4.4 Single Molecular Nuclear Spin Transistor

391

(2)

7.4.4.5 Molecule Based Hybrid Spintronic Devices

393

(2)

7.5 Electrochemistry with Nanogap Electrodes

395

(5)

References

400

(11)

Index

411

Tao Li is Associate Professor in the Department of Chemistry at Shanghai Jiao Tong University. His research interests are molecular electronics, molecular-scale devices, sythesis and application of organic functional materials and molecular solar thermal batteries.

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